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Get Free AccessKupfer oder Nickel? Der gezeigte CuII-Salen-Komplex, ein Modell des aktiven Zentrums der Galactose-Oxidase (GO), liegt im Festkörper als lokalisiertes Radikal vor, wie an der chinoiden Verteilung der Bindungslängen in einem der Ringe zu erkennen ist. Die Struktur des radikalischen Liganden hängt nicht vom Metall ab, die Zusammensetzung des SOMO dagegen schon. Dies könnte die viel geringere Reaktivität des Ni-Komplexes erklären, ebenso wie die Tatsache, dass natürliche GO ein CuII-Zentrum bevorzugt.
Maylis Orio, Olivier Jarjayes, Hussein Kanso, Christian Philouze, Frank Neese, Fabrice Thomas (2010). X‐Ray Structures of Copper(II) and Nickel(II) Radical Salen Complexes: The Preference of Galactose Oxidase for Copper(II). Angewandte Chemie, 122(29), pp. 5109-5112, DOI: 10.1002/ange.201001040.
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Type
Article
Year
2010
Authors
6
Datasets
0
Total Files
0
Language
German
Journal
Angewandte Chemie
DOI
10.1002/ange.201001040
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