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Get Free AccessA new type of ruthenium-based catalyst, labeled RuOxCy@C, consisting of a combination of metallic ruthenium (Ru0), ruthenium oxide (RuO2), and a ruthenium oxycarbonate phase (RuO2Cy) formed by interstitial carbon doped into RuO2, has been recently reported for low-temperature CO2 methanation. Its catalytic activity and long-term stability depend on two competing processes that take place under reaction conditions: RuO2 reduction with H2 to form inactive Ru0 nanoparticles, and C diffusion into RuO2 to form the active oxycarbonate phase. A combination of experimental and computational techniques is applied in this work to investigate the relative rate of both processes in order to identify possible modifications in the catalyst composition that might improve the overall catalytic performance.
Alvaro Royo de Larios, Carmen Tébar-Soler, Daviel Gómez, Patricia Concepción, Mercedes Boronat, Avelino Avelino (2025). Unlocking the Role of C Doping in a RuO<sub>2</sub> Matrix in CO<sub>2</sub> Methanation from a Combined Theoretical and Experimental Approach. The Journal of Physical Chemistry C, 129(11), pp. 5449-5460, DOI: 10.1021/acs.jpcc.5c01277.
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Type
Article
Year
2025
Authors
6
Datasets
0
Total Files
0
Language
English
Journal
The Journal of Physical Chemistry C
DOI
10.1021/acs.jpcc.5c01277
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