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Get Free AccessPt impregnated on a Sn-beta catalyst results in a very promising catalyst for the selective hydrogenation of α,β-unsaturated aldehydes, compared to the PtSn co-impregnated beta catalysts. Framework tin ions in the Sn-beta sample stabilize the nucleation of platinum nanoparticles inside the zeolite channel. These Pt0–Sn4+ sites, which are only observed in the Pt/Sn-beta catalyst, have been shown to strongly activate the carbonyl group enhancing the hydrogenation rate of the CO bond.
Patricia Concepción, Yolanda Pérez, Juan Carlos Hernández‐Garrido, Mariano Fajardo, José J. Calvino, Avelino Avelino (2013). The promotional effect of Sn-beta zeolites on platinum for the selective hydrogenation of α,β-unsaturated aldehydes. Physical Chemistry Chemical Physics, 15(29), pp. 12048-12048, DOI: 10.1039/c3cp50519g.
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Type
Article
Year
2013
Authors
6
Datasets
0
Total Files
0
Language
English
Journal
Physical Chemistry Chemical Physics
DOI
10.1039/c3cp50519g
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