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Get Free AccessThe structure of the oxygen-induced p(4 x 4) reconstruction of Ag(111) is determined by a combination of scanning tunneling microscopy, surface x-ray diffraction, core level spectroscopy, and density functional theory. We demonstrate that all previous models of this surface structure are incorrect and propose a new model which is able to explain all our experimental findings but has no resemblance to bulk silver oxide. We also shed some light on the limitations of current density functional theories and the potential role of van der Waals interactions in the stabilization of oxygen-induced surface reconstructions of noble metals.
Michael Schmid, A. Reicho, Andreas Stierle, I. Costina, J. Klikovits, Petr Kostelník, O. Dubay, Kresse Georg, Johan Gustafson, Edvin Lundgren, J. N. Andersen, H. Dosch, П. Варга (2006). Structure of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>Ag</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mn>111</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext mathvariant="normal">−</mml:mtext><mml:mi>p</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mn>4</mml:mn><mml:mo>×</mml:mo><mml:mn>4</mml:mn><mml:mo stretchy="false">)</mml:mo><mml:mtext mathvariant="normal">−</mml:mtext><mml:mi mathvariant="normal">O</mml:mi></mml:math>: No Silver Oxide. Physical Review Letters, 96(14), DOI: 10.1103/physrevlett.96.146102.
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Type
Article
Year
2006
Authors
13
Datasets
0
Total Files
0
Language
English
Journal
Physical Review Letters
DOI
10.1103/physrevlett.96.146102
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