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Get Free AccessTwo strategies to improve the catalytic activity of Ti-MCM-41 materials in the epoxidation of olefins are described; the first approach involves silylation of the surface of Ti-MCM-41 which produces a very hydrophobic catalyst whereas the second approach is based on removal of water from the reaction media; the increase in activity is not due to a change in the intrinsic activity of the Ti sites, but rather to a decrease of the catalyst deactivation by reducing the formation of diols produced by ring opening of the epoxide.
Avelino Avelino, Marcelo E. Domine, J.A. López Gaona, J.L. Jordá, M. Navarro, Fernando Rey, Joaquín Pérez‐Pariente, Junpei Tsuji, Beth McCulloch, László Németh (1998). Strategies to improve the epoxidation activity and selectivity of Ti-MCM-41. Chemical Communications, pp. 2211-2212, DOI: 10.1039/a806702c.
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Type
Article
Year
1998
Authors
10
Datasets
0
Total Files
0
Language
English
Journal
Chemical Communications
DOI
10.1039/a806702c
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