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Get Free AccessThe electronic band gap of a two-dimensional semiconductor within a device architecture is sensitive to variations in screening properties of adjacent materials in the device and to gate-controlled doping. Here, we employ microfocused angle-resolved photoemission spectroscopy to separate band gap renormalization effects stemming from environmental screening and electron doping during in situ gating of a single-layer WS_{2} device. The WS_{2} is supported on hexagonal boron nitride and contains a section that is exposed to vacuum and another section that is encapsulated by a graphene contact. We directly observe the doping-induced semiconductor-metal transition and band gap renormalization in the two sections of WS_{2}. Surprisingly, a larger band gap renormalization is observed in the vacuum-exposed section than in the graphene-encapsulated-and thus ostensibly better screened-section of the WS_{2}. Using GW calculations, we determine that intrinsic screening due to stronger doping in vacuum-exposed WS_{2} exceeds the external environmental screening in graphene-encapsulated WS_{2}.
Yann in ’t Veld, Alfred J. H. Jones, Zhihao Jiang, Greta Lupi, Paulina Majchrzak, Kimberly Hsieh, Kenji Watanabe, Takashi Taniguchi, Philip Hofmann, Jill A. Miwa, Yong P. Chen, Malte Rösner, Søren Ulstrup (2025). Quasiparticle Gap Renormalization Driven by Internal and External Screening in a <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>WS</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Device. , 135(5), DOI: https://doi.org/10.1103/yllv-5zx7.
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Type
Article
Year
2025
Authors
13
Datasets
0
Total Files
0
Language
lv
DOI
https://doi.org/10.1103/yllv-5zx7
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