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Get Free AccessA combination of Photoemission, Atomic Force and Scanning Tunneling Microscopy/Spectroscopy measurements shows that excess electrons in TiO2 anatase (101) surface are trapped at step edges. Consequently, steps act as preferred adsorption sites for O2. In Density Functional Theory calculations electrons localize at clean step edges, this tendency is enhanced by O vacancies and hydroxylation. The results show the importance of defects for the wide-ranging applications of titania.
Martin Setvín, Xianfeng Hao, Benjamin Daniel, Jiří Pavelec, Zbyněk Novotný, Gareth S. Parkinson, Michael Schmid, Kresse Georg, Cesare Franchini, Ulrike Diebold (2014). Charge Trapping at the Step Edges of TiO<sub>2</sub> Anatase (101). Angewandte Chemie International Edition, 53(18), pp. 4714-4716, DOI: 10.1002/anie.201309796.
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Type
Article
Year
2014
Authors
10
Datasets
0
Total Files
0
Language
English
Journal
Angewandte Chemie International Edition
DOI
10.1002/anie.201309796
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