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Get Free AccessIn the hydrothermal crystallization of zeolites from basic media, hydroxide ions (OH(-)) catalyze the depolymerization of the aluminosilicate gel by breaking the Si,Al-O-Si,Al bonds and catalyze the polymerization of the aluminosilicate anions around the hydrated cation species by remaking the Si,Al-O-Si,Al bonds. We report that hydroxyl free radicals (•OH) are involved in the zeolite crystallization under hydrothermal conditions. The crystallization processes of zeolites-such as Na-A, Na-X, NaZ-21, and silicalite-1-can be accelerated with hydroxyl free radicals generated by ultraviolet irradiation or Fenton's reagent.
Guodong Feng, Peng Cheng, Wenfu Yan, Mercedes Boronat, Xu Li, Ji‐Hu Su, Jianyu Wang, Yi Li, Avelino Avelino, Ruren Xu, Jihong Yu (2016). Accelerated crystallization of zeolites via hydroxyl free radicals. Science, 351(6278), pp. 1188-1191, DOI: 10.1126/science.aaf1559.
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Type
Article
Year
2016
Authors
11
Datasets
0
Total Files
0
Language
English
Journal
Science
DOI
10.1126/science.aaf1559
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